Seasonal variations and sources of atmospheric polycyclic aromatic hydrocarbons and organochlorine compounds in a high-altitude city: Evidence from four-year observations | |
Gong, P (Gong, Ping)1,2; Wang, XP (Wang, Xiaoping)1,2; Sheng, JJ (Sheng, Jiujiang)1; Wang, HL (Wang, Hailong)3; Yuan, XH (Yuan, Xiaohua)1; He, YQ (He, Yuanqing)4; Qian, Y (Qian, Yun)3; Yao, TD (Yao, Tandong)1,2 | |
刊名 | ENVIRONMENTAL POLLUTION |
2018-02-01 | |
卷号 | 233期号:0页码:1188-1197 |
关键词 | LONG-RANGE TRANSPORT NORTH PACIFIC-OCEAN PERSISTENT ORGANIC POLLUTANTS SOUTHEAST TIBETAN PLATEAU ADJACENT ARCTIC REGION POLYCHLORINATED-BIPHENYLS SOURCE APPORTIONMENT SPATIAL-DISTRIBUTION LHASA CITY CARBONACEOUS AEROSOLS |
ISSN号 | 0269-7491 |
DOI | 10.1016/j.envpol.2017.10.064 |
英文摘要 | Lijiang is a high-altitude city located on the eastern fringe of the Tibetan Plateau, with complex seasonal atmospheric circulaticins (i.e. westerly wind, Indian Monsoon, and East Asia Monsoon). Very few previous studies have focused on seasonal variations and sources of organic pollutants in Lijiang. In this study, a four-year air campaign from June 2009 to July 2013 was conducted to investigate the temporal trends and the sources of polycyclic aromatic hydrocarbons (PAHs) and organochlorine compounds [including organochlorine pesticides (OCPs) and polychlorinated biphenyls (PCBs)]. The atmospheric PAH concentrations in winter are 2-3 times of those in summer, probably because of the combined result of enhanced local emission and long-range atmospheric transport (LRAT) during winter. Traffic pollution was the primary local source of PAHs, while biomass burning is the dominant LRAT source. OCPs and PCBs also mainly underwent LRAT to reach Lijiang. The peak concentrations of most of OCPs occurred in pre-monsoon season and winter, which were carried by air masses from Myanmar and India through westerly winds. As compared with other sites of the Tibetan Plateau, without the direct barrier of the Himalaya, Lijiang is easily contaminated by the incursion of polluted air masses. (C) 2017 Elsevier Ltd. All rights reserved. |
WOS研究方向 | Environmental Sciences & Ecology |
语种 | 英语 |
出版者 | ELSEVIER SCI LTD |
WOS记录号 | WOS:000424177000126 |
内容类型 | 期刊论文 |
源URL | [http://ir.itpcas.ac.cn/handle/131C11/8744] |
专题 | 青藏高原研究所_图书馆 |
作者单位 | 1.Chinese Acad Sci, Inst Tibetan Plateau Res, Key Lab Tibetan Environm Changes & Land Surface P, Beijing 100101, Peoples R China; 2.CAS Ctr Excellence Tibetan Plateau Earth Sci, Beijing 100101, Peoples R China; 3.PNNL, Atmospher Sci & Global Change Div, Richland, WA 99352 USA; 4.Chinese Acad Sci, Northwest Inst Ecoenvironm & Resources, State Key Lab Cryosphere Sci, Lanzhou 730000, Gansu, Peoples R China. |
推荐引用方式 GB/T 7714 | Gong, P ,Wang, XP ,Sheng, JJ ,et al. Seasonal variations and sources of atmospheric polycyclic aromatic hydrocarbons and organochlorine compounds in a high-altitude city: Evidence from four-year observations[J]. ENVIRONMENTAL POLLUTION,2018,233(0):1188-1197. |
APA | Gong, P .,Wang, XP .,Sheng, JJ .,Wang, HL .,Yuan, XH .,...&Yao, TD .(2018).Seasonal variations and sources of atmospheric polycyclic aromatic hydrocarbons and organochlorine compounds in a high-altitude city: Evidence from four-year observations.ENVIRONMENTAL POLLUTION,233(0),1188-1197. |
MLA | Gong, P ,et al."Seasonal variations and sources of atmospheric polycyclic aromatic hydrocarbons and organochlorine compounds in a high-altitude city: Evidence from four-year observations".ENVIRONMENTAL POLLUTION 233.0(2018):1188-1197. |
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