Reconstruction of the Wet Chemical Synthesis Process: The Case of Fe5C2 Nanoparticles

doi:10.1021/acs.jpcc.7b00198

	Reconstruction of the Wet Chemical Synthesis Process: The Case of Fe5C2 Nanoparticles
	Li, Siwei 2; Yao, Siyu 2; Yang, Ce 1,2; Zhao, Huabo 2; Lin, Lili 2; Wen, Wen 3; Liu, Jinxun 4,5; Hu, Gang 6; Li, Weixue 4,5; Hou, Yanglong 1
刊名	JOURNAL OF PHYSICAL CHEMISTRY C
	2017-03-09
卷号	121 期号:9 页码:5154-5160
ISSN号	1932-7447
DOI	10.1021/acs.jpcc.7b00198
文献子类	Article
英文摘要	Wet chemical synthesis (WCS), especially under high temperatures, is one of the most frequently used strategies for nanostructured material construction, which has been used extensively in medical-, energy-, and environment-related applications. Although knowledge about the WCS process has been accumulated in the past two decades, the high temperature used in the process and multiphase nature of intermediates and products are key factors preventing the processes from rationalization. In this paper, by using multilevel in situ cells, we developed a strategy to monitor the reaction details of WCS processed in the solid, liquid, and gas phase simultaneously. This protocol has proven successful to reconstruct the WCS process of Fe5C2 nanoparticles (NPs) and unravel the complicated chemistry in the synthesis process.
WOS关键词	FISCHER-TROPSCH SYNTHESIS ; IRON CARBIDE NANOPARTICLES ; MINIMUM ENERGY PATHS ; ELASTIC BAND METHOD ; X-RAY-SCATTERING ; HYDROTHERMAL CONDITIONS ; SYNCHROTRON-RADIATION ; NANOCOMPOSITE MAGNETS ; COBALT NANOPARTICLES ; GRAPHITIC LAYERS
WOS研究方向	Chemistry ; Science & Technology - Other Topics ; Materials Science
语种	英语
出版者	AMER CHEMICAL SOC
WOS记录号	WOS:000396295800041
内容类型	期刊论文
源URL	[http://cas-ir.dicp.ac.cn/handle/321008/169414]
专题	大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者	Hou, Yanglong; Ma, Ding
作者单位	1.Peking Univ, Coll Engn, Beijing 100871, Peoples R China 2.Peking Univ, Coll Chem & Mol Engn, Beijing 100871, Peoples R China 3.Chinese Acad Sci, Shanghai Inst Appl Phys, SSRF, Shanghai 201204, Peoples R China 4.Univ Sci & Technol China, Dept Chem Phys, Hefei 230026, Peoples R China 5.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China 6.Israel Chem Ltd, Shanghai 200021, Peoples R China
推荐引用方式 GB/T 7714	Li, Siwei,Yao, Siyu,Yang, Ce,et al. Reconstruction of the Wet Chemical Synthesis Process: The Case of Fe5C2 Nanoparticles[J]. JOURNAL OF PHYSICAL CHEMISTRY C,2017,121(9):5154-5160.
APA	Li, Siwei.,Yao, Siyu.,Yang, Ce.,Zhao, Huabo.,Lin, Lili.,...&Ma, Ding.(2017).Reconstruction of the Wet Chemical Synthesis Process: The Case of Fe5C2 Nanoparticles.JOURNAL OF PHYSICAL CHEMISTRY C,121(9),5154-5160.
MLA	Li, Siwei,et al."Reconstruction of the Wet Chemical Synthesis Process: The Case of Fe5C2 Nanoparticles".JOURNAL OF PHYSICAL CHEMISTRY C 121.9(2017):5154-5160.