Continuous Synthesis of Ag/AgCl/ZnO Composites Using Flow Chemistry and Photocatalytic Application

doi:10.1021/acs.iecr.7b05263

	Continuous Synthesis of Ag/AgCl/ZnO Composites Using Flow Chemistry and Photocatalytic Application
	Tao, Sha 1,2; Yang, Mei 2; Chen, Huihui 1,2; Zhao, Shuainan 1,2; Chen, Guangwen 2
刊名	INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
	2018-03-07
卷号	57 期号:9 页码:3263-3273
ISSN号	0888-5885
DOI	10.1021/acs.iecr.7b05263
文献子类	Article
英文摘要	Ag/AgCl/ZnO composites were successfully synthesized in a continuous microfluidic system under visible light irradiation, which was employed in situ to reduce a portion of AgCl to metallic Ag. The formation of Ag/AgCl/ZnO composites was confined in small aqueous plugs, which were dispersed by octane as the continuous phase. In this way, enhanced mixing, low risk of channel clogging, and uniform light distribution were achieved. The characterization results revealed that the as-prepared Ag/AgCl/ZnO composites were composed of flowerlike ZnO with Ag/AgCl nanospheres anchored to them. It was found that the synthesis parameters such as water/oil volume flow ratio, total volume flow rate, temperature, and the molar ratio of Zn2+ to Ag+ had effects on the synthesis of Ag/AgCl/ZnO composites. Furthermore, the as-prepared Ag/AgCl/ZnO composites outperformed Ag/ZnO composites and AgCl/ZnO composites in the visible-light-driven degradation of methyl orange.
WOS关键词	AG-AT-AGCL ; ASSESSING MICROMIXING EFFICIENCY ; SURFACE-PLASMON RESONANCE ; COMPETING REACTION SYSTEM ; LIQUID SLUG FLOW ; VISIBLE-LIGHT ; HIGHLY EFFICIENT ; SEGMENTED FLOW ; NANOPARTICLE SYNTHESIS ; FACILE SYNTHESIS
WOS研究方向	Engineering
语种	英语
出版者	AMER CHEMICAL SOC
WOS记录号	WOS:000427203000015
内容类型	期刊论文
源URL	[http://cas-ir.dicp.ac.cn/handle/321008/168916]
专题	大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者	Yang, Mei; Chen, Guangwen
作者单位	1.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China
推荐引用方式 GB/T 7714	Tao, Sha,Yang, Mei,Chen, Huihui,et al. Continuous Synthesis of Ag/AgCl/ZnO Composites Using Flow Chemistry and Photocatalytic Application[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2018,57(9):3263-3273.
APA	Tao, Sha,Yang, Mei,Chen, Huihui,Zhao, Shuainan,&Chen, Guangwen.(2018).Continuous Synthesis of Ag/AgCl/ZnO Composites Using Flow Chemistry and Photocatalytic Application.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,57(9),3263-3273.
MLA	Tao, Sha,et al."Continuous Synthesis of Ag/AgCl/ZnO Composites Using Flow Chemistry and Photocatalytic Application".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 57.9(2018):3263-3273.