Coherent interference of molecular electronic states in NO by two-color femtosecond laser pulses

doi:10.1103/PhysRevA.99.011402

	Coherent interference of molecular electronic states in NO by two-color femtosecond laser pulses
	Ding, Dajun 2; Sun, Zhigang 1; Yuan, Kai-Jun 2,3; Bandrauk, Andre D.3; Hu, Wenhui 2; Liu, Yong 1; Luo, Sizuo 2; Li, Xing 2; Yu, Jiaqi 2; Li, Xiaokai 2
刊名	PHYSICAL REVIEW A
	2019-01-22
卷号	99 期号:1 页码:6
ISSN号	2469-9926
DOI	10.1103/PhysRevA.99.011402
通讯作者	Luo, Sizuo(luosz@jlu.edu.cn) ; Yuan, Kai-Jun(kaijun.yuan@usherbrooke.ca) ; Ding, Dajun(dajund@jlu.edu.cn)
英文摘要	Quantum coherence interference between electronic states in molecules is an important factor for controlling electronic and nuclear dynamics in photoinduced physics and chemistry. We measure and model molecular angle-dependent photoionization yields to explore coherent interference dynamics between quasiequal energy electronic-vibrational states of the nitric oxide molecule, NO, by ultrafast phase-controlled two-color femtosecond laser pulses. We demonstrate by experiment and theory that the photoelectron angular distribution of NO, where two excited electronic states are coherently combined by ultrafast pulses, is a function of the relative phase of the pulses, and the photoelectron kinetic energy. The modification of photoelectron emission angular patterns encodes the information of the coherence via electronic state interference. The result allows access to phase-dependent state correlations and ultrafast vibrationic dynamics in molecules.
资助项目	National Natural Science Foundation of China (NNSFC)[11704148] ; National Natural Science Foundation of China (NNSFC)[11534004] ; National Natural Science Foundation of China (NNSFC)[11627807] ; National Natural Science Foundation of China (NNSFC)[21222308] ; National Natural Science Foundation of China (NNSFC)[21133006] ; National Natural Science Foundation of China (NNSFC)[21433009] ; China Postdoctoral Science Foundation[2015M571336] ; NSERC ; FQRNT
WOS关键词	CIRCULAR-DICHROISM ; DYNAMICS ; PHOTOELECTRON ; DIFFRACTION ; IONIZATION ; MIGRATION ; BREAKING
WOS研究方向	Optics ; Physics
语种	英语
出版者	AMER PHYSICAL SOC
WOS记录号	WOS:000456287500003
资助机构	National Natural Science Foundation of China (NNSFC) ; National Natural Science Foundation of China (NNSFC) ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; NSERC ; NSERC ; FQRNT ; FQRNT ; National Natural Science Foundation of China (NNSFC) ; National Natural Science Foundation of China (NNSFC) ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; NSERC ; NSERC ; FQRNT ; FQRNT ; National Natural Science Foundation of China (NNSFC) ; National Natural Science Foundation of China (NNSFC) ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; NSERC ; NSERC ; FQRNT ; FQRNT ; National Natural Science Foundation of China (NNSFC) ; National Natural Science Foundation of China (NNSFC) ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; NSERC ; NSERC ; FQRNT ; FQRNT
内容类型	期刊论文
源URL	[http://cas-ir.dicp.ac.cn/handle/321008/166292]
专题	大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者	Ding, Dajun; Yuan, Kai-Jun; Luo, Sizuo
作者单位	1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China 2.Jilin Univ, Inst Atom & Mol Phys, Changchun 130012, Jilin, Peoples R China 3.Univ Sherbrooke, Fac Sci, Lab Chim Theor, Sherbrooke, PQ J1K 2R1, Canada
推荐引用方式 GB/T 7714	Ding, Dajun,Sun, Zhigang,Yuan, Kai-Jun,et al. Coherent interference of molecular electronic states in NO by two-color femtosecond laser pulses[J]. PHYSICAL REVIEW A,2019,99(1):6.
APA	Ding, Dajun.,Sun, Zhigang.,Yuan, Kai-Jun.,Bandrauk, Andre D..,Hu, Wenhui.,...&Li, Xiaokai.(2019).Coherent interference of molecular electronic states in NO by two-color femtosecond laser pulses.PHYSICAL REVIEW A,99(1),6.
MLA	Ding, Dajun,et al."Coherent interference of molecular electronic states in NO by two-color femtosecond laser pulses".PHYSICAL REVIEW A 99.1(2019):6.