Dynamical interference in the vibronic bond breaking reaction of HCO

doi:10.1126/sciadv.aau0582

	Dynamical interference in the vibronic bond breaking reaction of HCO
	Han, Shanyu 2,3; Zheng, Xianfeng 1,4; Ndengue, Steve 5; Song, Yu 1; Dawes, Richard 5; Xie, Daiqian 2,6,7,8; Zhang, Jingsong 1; Guo, Hua 3
刊名	SCIENCE ADVANCES
	2019
卷号	5 期号:1 页码:6
ISSN号	2375-2548
DOI	10.1126/sciadv.aau0582
通讯作者	Dawes, Richard(dawesr@mst.edu) ; Xie, Daiqian(dqxie@nju.edu.cn) ; Zhang, Jingsong(jingsong.zhang@ucr.edu) ; Guo, Hua(hguo@unm.edu)
英文摘要	First-principles treatments of quantum molecular reaction dynamics have reached the level of quantitative accuracy even in cases with strong non-Born-Oppenheimer effects. This achievement permits the interpretation of puzzling experimental phenomena related to dynamics governed by multiple coupled potential energy surfaces. We present a combined experimental and theoretical study of the photodissociation of formyl radical (HCO). Oscillations observed in the distribution of product states are found to arise from the interference of matter waves-a manifestation analogous to Young's double-slit experiment.
资助项目	National Natural Science Foundation of China[21688102] ; National Natural Science Foundation of China[21733006] ; National Natural Science Foundation of China[21590802] ; National Key Research and Development Program of China[2017YFA0206500] ; NSF[CHE-1566636] ; U.S. Department of Energy Office of Science, Office of Basic Energy Sciences[DE-SC0010616] ; U.S. Department of Energy Office of Science, Office of Basic Energy Sciences[DE-SC0015997]
WOS关键词	STATE PHOTODISSOCIATION DYNAMICS ; POTENTIAL-ENERGY SURFACE ; 1ST ABSORPTION-BAND ; RENNER-TELLER ; AB-INITIO ; UNIMOLECULAR DISSOCIATION ; TRIATOMIC-MOLECULES ; DISTRIBUTIONS ; SPECTROSCOPY ; TRANSITION
WOS研究方向	Science & Technology - Other Topics
语种	英语
出版者	AMER ASSOC ADVANCEMENT SCIENCE
WOS记录号	WOS:000457547900003
资助机构	National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; NSF ; NSF ; U.S. Department of Energy Office of Science, Office of Basic Energy Sciences ; U.S. Department of Energy Office of Science, Office of Basic Energy Sciences ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; NSF ; NSF ; U.S. Department of Energy Office of Science, Office of Basic Energy Sciences ; U.S. Department of Energy Office of Science, Office of Basic Energy Sciences ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; NSF ; NSF ; U.S. Department of Energy Office of Science, Office of Basic Energy Sciences ; U.S. Department of Energy Office of Science, Office of Basic Energy Sciences ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; NSF ; NSF ; U.S. Department of Energy Office of Science, Office of Basic Energy Sciences ; U.S. Department of Energy Office of Science, Office of Basic Energy Sciences
内容类型	期刊论文
源URL	[http://cas-ir.dicp.ac.cn/handle/321008/166076]
专题	大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者	Dawes, Richard; Xie, Daiqian; Zhang, Jingsong; Guo, Hua
作者单位	1.Univ Calif Riverside, Dept Chem, Riverside, CA 92521 USA 2.Nanjing Univ, Sch Chem & Chem Engn, Key Lab Mesoscop Chem, Inst Theoret & Computat Chem, Nanjing 210093, Jiangsu, Peoples R China 3.Univ New Mexico, Dept Chem & Chem Biol, Albuquerque, NM 87131 USA 4.Anhui Normal Univ, Dept Phys, Anhui Prov Key Lab Optoelect Mat Sci & Technol, Wuhu 241000, Anhui, Peoples R China 5.Missouri Univ Sci & Technol, Dept Chem, Rolla, MO 65409 USA 6.Univ Sci & Technol China, Synerget Innovat Ctr Quantum Informat & Quantum P, Hefei 230026, Anhui, Peoples R China 7.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China 8.Chinese Acad Sci, Dalian Inst Chem Phys, Ctr Theoret Computat Chem, Dalian 116023, Peoples R China
推荐引用方式 GB/T 7714	Han, Shanyu,Zheng, Xianfeng,Ndengue, Steve,et al. Dynamical interference in the vibronic bond breaking reaction of HCO[J]. SCIENCE ADVANCES,2019,5(1):6.
APA	Han, Shanyu.,Zheng, Xianfeng.,Ndengue, Steve.,Song, Yu.,Dawes, Richard.,...&Guo, Hua.(2019).Dynamical interference in the vibronic bond breaking reaction of HCO.SCIENCE ADVANCES,5(1),6.
MLA	Han, Shanyu,et al."Dynamical interference in the vibronic bond breaking reaction of HCO".SCIENCE ADVANCES 5.1(2019):6.