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Functionalised heterogeneous catalysts for sustainable biomass valorisation
Sudarsanam, Putla1; Zhong, Ruyi2,3; Van den Bosch, Sander1; Coman, Simona M.4; Parvulescu, Vasile I.4; Sels, Bert F.1
刊名Chemical society reviews
2018-11-21
卷号47期号:22页码:8349-8402
ISSN号0306-0012
DOI10.1039/c8cs00410b
通讯作者Sudarsanam, putla(sudarsanam.putla@kuleuven.be) ; Parvulescu, vasile i.() ; Sels, bert f.(bert.sels@biw.kuleuven.be)
英文摘要Efficient transformation of biomass to value-added chemicals and high-energy density fuels is pivotal for a more sustainable economy and carbon-neutral society. in this framework, developing potential cascade chemical processes using functionalised heterogeneous catalysts is essential because of their versatile roles towards viable biomass valorisation. advances in materials science and catalysis have provided several innovative strategies for the design of new appealing catalytic materials with well-defined structures and special characteristics. promising catalytic materials that have paved the way for exciting scientific breakthroughs in biomass upgrading are carbon materials, metal-organic frameworks, solid phase ionic liquids, and magnetic iron oxides. these fascinating catalysts offer unique possibilities to accommodate adequate amounts of acid-base and redox functional species, hence enabling various biomass conversion reactions in a one-pot way. this review therefore aims to provide a comprehensive account of the most significant advances in the development of functionalised heterogeneous catalysts for efficient biomass upgrading. in addition, this review highlights important progress ensued in tailoring the immobilisation of desirable functional groups on particular sites of the above-listed materials, while critically discussing the role of consequent properties on cascade reactions as well as on other vital processes within the bio-refinery. current challenges and future opportunities towards a rational design of novel functionalised heterogeneous catalysts for sustainable biomass valorisation are also emphasized.
WOS关键词METAL-ORGANIC FRAMEWORKS ; SOLID ACID CATALYST ; SELECTIVE AEROBIC OXIDATION ; SUPPORTED IONIC LIQUIDS ; CARBON-BASED CATALYST ; GRAPHENE OXIDE CATALYSTS ; WASTE COOKING OIL ; MAGNETICALLY RECOVERABLE NANOCATALYSTS ; BIO-ADDITIVE FUELS ; ONE-POT CONVERSION
WOS研究方向Chemistry
WOS类目Chemistry, Multidisciplinary
语种英语
出版者ROYAL SOC CHEMISTRY
WOS记录号WOS:000449968700006
内容类型期刊论文
URI标识http://www.corc.org.cn/handle/1471x/2373112
专题大连化学物理研究所
通讯作者Sudarsanam, Putla; Parvulescu, Vasile I.; Sels, Bert F.
作者单位1.Katholieke Univ Leuven, Fac Biosci Engn, Ctr Surface Chem & Catalysis, Celestijnenlaan 200f, B-3001 Heverlee, Belgium
2.Southern Univ Sci & Technol, Dept Chem, Shenzhen 518055, Peoples R China
3.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
4.Univ Bucharest, Dept Organ Chem Biochem & Catalysis, Bdul Regina Elisabeta 4-12, Bucharest 030016, Romania
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GB/T 7714
Sudarsanam, Putla,Zhong, Ruyi,Van den Bosch, Sander,et al. Functionalised heterogeneous catalysts for sustainable biomass valorisation[J]. Chemical society reviews,2018,47(22):8349-8402.
APA Sudarsanam, Putla,Zhong, Ruyi,Van den Bosch, Sander,Coman, Simona M.,Parvulescu, Vasile I.,&Sels, Bert F..(2018).Functionalised heterogeneous catalysts for sustainable biomass valorisation.Chemical society reviews,47(22),8349-8402.
MLA Sudarsanam, Putla,et al."Functionalised heterogeneous catalysts for sustainable biomass valorisation".Chemical society reviews 47.22(2018):8349-8402.
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