CORC  > 大连化学物理研究所
Coherent interference of molecular electronic states in no by two-color femtosecond laser pulses
Hu, Wenhui1; Liu, Yong2; Luo, Sizuo1; Li, Xing1; Yu, Jiaqi1; Li, Xiaokai1; Sun, Zhigang2; Yuan, Kai-Jun1,3; Bandrauk, Andre D.3; Ding, Dajun1
刊名Physical review a
2019-01-22
卷号99期号:1页码:6
ISSN号2469-9926
DOI10.1103/physreva.99.011402
通讯作者Luo, sizuo(luosz@jlu.edu.cn) ; Yuan, kai-jun(kaijun.yuan@usherbrooke.ca) ; Ding, dajun(dajund@jlu.edu.cn)
英文摘要Quantum coherence interference between electronic states in molecules is an important factor for controlling electronic and nuclear dynamics in photoinduced physics and chemistry. we measure and model molecular angle-dependent photoionization yields to explore coherent interference dynamics between quasiequal energy electronic-vibrational states of the nitric oxide molecule, no, by ultrafast phase-controlled two-color femtosecond laser pulses. we demonstrate by experiment and theory that the photoelectron angular distribution of no, where two excited electronic states are coherently combined by ultrafast pulses, is a function of the relative phase of the pulses, and the photoelectron kinetic energy. the modification of photoelectron emission angular patterns encodes the information of the coherence via electronic state interference. the result allows access to phase-dependent state correlations and ultrafast vibrationic dynamics in molecules.
WOS关键词CIRCULAR-DICHROISM ; DYNAMICS ; PHOTOELECTRON ; DIFFRACTION ; IONIZATION ; MIGRATION ; BREAKING
WOS研究方向Optics ; Physics
WOS类目Optics ; Physics, Atomic, Molecular & Chemical
语种英语
出版者AMER PHYSICAL SOC
WOS记录号WOS:000456287500003
内容类型期刊论文
URI标识http://www.corc.org.cn/handle/1471x/2372910
专题大连化学物理研究所
通讯作者Luo, Sizuo; Yuan, Kai-Jun; Ding, Dajun
作者单位1.Jilin Univ, Inst Atom & Mol Phys, Changchun 130012, Jilin, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
3.Univ Sherbrooke, Fac Sci, Lab Chim Theor, Sherbrooke, PQ J1K 2R1, Canada
推荐引用方式
GB/T 7714
Hu, Wenhui,Liu, Yong,Luo, Sizuo,et al. Coherent interference of molecular electronic states in no by two-color femtosecond laser pulses[J]. Physical review a,2019,99(1):6.
APA Hu, Wenhui.,Liu, Yong.,Luo, Sizuo.,Li, Xing.,Yu, Jiaqi.,...&Ding, Dajun.(2019).Coherent interference of molecular electronic states in no by two-color femtosecond laser pulses.Physical review a,99(1),6.
MLA Hu, Wenhui,et al."Coherent interference of molecular electronic states in no by two-color femtosecond laser pulses".Physical review a 99.1(2019):6.
个性服务
查看访问统计
相关权益政策
暂无数据
收藏/分享
所有评论 (0)
暂无评论
 

除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。


©版权所有 ©2017 CSpace - Powered by CSpace