Promising application of SiC without co-catalyst in photocatalysis and ozone integrated process for aqueous organics degradation | |
Xie, YB; Yan, J; Chen, Y; Liu, XL; Zhao, H; Yao, YJ; Cao, HB; Xie, Yongbing; Yan, Jin; Chen, Yue | |
刊名 | CATALYSIS TODAY |
2018 | |
卷号 | 315页码:223 |
关键词 | SiC VISIBLE-LIGHT-DRIVEN Photocatalytic ozonation HYDROGEN-PRODUCTION Penicilin G SILICON-CARBIDE Band structure H-2 EVOLUTION Reaction mechanism WASTE-WATER OZONATION SURFACE OXIDATION COMPOSITES CATALYSTS |
ISSN号 | 0920-5861 |
DOI | 10.1016/j.cattod.2018.01.013 |
文献子类 | Article |
英文摘要 | SiC is a newly developed photocatalyst, but it is often used together with a co-catalyst rather than solely for its relatively low activity. Here we reported the high activity of a commercial SiC in a photocatalysis and ozone combined process (photocatalytic ozonation). The commercial SiC showed very weak activity in photocatalysis of oxalic acid (OA) and para-hydroxybenzoic acid (PHBA) degradation, and its performance in catalytic ozonation was also not satisfied. However, the organics degradation and mineralization rates dramatically increased in the SiC photocatalytic ozonation. The different operation parameters were optimized, and the main reactive radicals in this process and its generation pathways were studied. It was found that photo-generated electron reduction of ozone and oxygen are the main pathways to produce hydroxyl radical, which was responsible to the high oxidizing ability of this process. |
WOS记录号 | WOS:000438466000025 |
内容类型 | 期刊论文 |
源URL | [http://ir.ipe.ac.cn/handle/122111/26699] |
专题 | 中国科学院过程工程研究所 |
推荐引用方式 GB/T 7714 | Xie, YB,Yan, J,Chen, Y,et al. Promising application of SiC without co-catalyst in photocatalysis and ozone integrated process for aqueous organics degradation[J]. CATALYSIS TODAY,2018,315:223, 229. |
APA | Xie, YB.,Yan, J.,Chen, Y.,Liu, XL.,Zhao, H.,...&Cao, Hongbin.(2018).Promising application of SiC without co-catalyst in photocatalysis and ozone integrated process for aqueous organics degradation.CATALYSIS TODAY,315,223. |
MLA | Xie, YB,et al."Promising application of SiC without co-catalyst in photocatalysis and ozone integrated process for aqueous organics degradation".CATALYSIS TODAY 315(2018):223. |
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