Facile synthesis of PEI-GO@ZIF-8 hybrid material for CO2 capture | |
Feng, Bo; Huang, Aisheng | |
刊名 | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY |
2018 | |
卷号 | 43期号:4页码:2224-2231 |
关键词 | Metal-organic Framework Zeolitic Imidazolate Framework Graphene Oxide Membranes Mixed-matrix Membranes Carbon-dioxide Capture In-situ Synthesis 3-dimensional Graphene Hydrogen Selectivity Seawater Desalination Co2/ch4 Separation |
英文摘要 | Pristine graphene oxide (GO) sheets were pretreated with polyethyleneimine (PEI) to prepare PEI-modified GO (PEI-GO), which was further inserted with ZIF-8 crystals to form a novel PEI-GO@ZIF-8 nanocomposite for CO2 capture. The good dispersion of PEI and interlayer growth of ZIF-8 within the GO sheets is helpful for high CO2 adsorption. Therefore, the PEI-GO@ZIF-8 nanocomposite show high surface area and enhanced CO2 adsorption capacity. The adsorption capacity of the PEI-GO@ZIF-8 nanocomposite was six times higher than that of the pristine GO and ZIF-8. The CO2/N-2 adsorption selectivity was significantly improved due to amine groups loading which provide more sites for CO2 adsorption. The preferential adsorption of CO2 over N-2 makes PEI-GO@ZIF-8 nano composite be a promising candidate in the field of CO2 capture. (C) 2017 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved. |
学科主题 | Chemistry ; Food Science & Technology ; Spectroscopy |
语种 | 英语 |
公开日期 | 2018-12-04 |
内容类型 | 期刊论文 |
源URL | [http://ir.nimte.ac.cn/handle/174433/16859] |
专题 | 2018专题 |
推荐引用方式 GB/T 7714 | Feng, Bo,Huang, Aisheng. Facile synthesis of PEI-GO@ZIF-8 hybrid material for CO2 capture[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2018,43(4):2224-2231. |
APA | Feng, Bo,&Huang, Aisheng.(2018).Facile synthesis of PEI-GO@ZIF-8 hybrid material for CO2 capture.INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,43(4),2224-2231. |
MLA | Feng, Bo,et al."Facile synthesis of PEI-GO@ZIF-8 hybrid material for CO2 capture".INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 43.4(2018):2224-2231. |
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