Characterization of Primary Organic Aerosol from Domestic Wood, Peat, and Coal Burning in Ireland

doi:10.1021/acs.est.7b01926

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	Characterization of Primary Organic Aerosol from Domestic Wood, Peat, and Coal Burning in Ireland
	O'Dowd, Colin 2,7; Huang, Ru-Jin 1,2,3,4,7; Prevot, Andre Stephan Henry 1; Canonaco, Francesco 1; Lin, Chunshui 2,3,4,7; Ceburnis, Darius 2,7; Hellebust, Stig 5,6; Buckley, Paul 5,6; Wenger, John 5,6; Ovadnevaite, Jurgita 2,7
刊名	ENVIRONMENTAL SCIENCE & TECHNOLOGY
	2017-09-19
卷号	51 期号:18 页码:10624-10632
DOI	10.1021/acs.est.7b01926
文献子类	Article
英文摘要	An aerosol chemical speciation monitor (ACSM) was deployed to study the primary nonrefractory submicron particulate matter emissions from the burning of commercially available solid fuels (peat, coal, and wood) typically used in European domestic fuel stoves. Organic mass spectra (MS) from burning wood, peat, and coal were characterized and intercompared for factor analysis against ambient data. The reference profiles characterized in this study were used to estimate the contribution of solid fuel sources, along with oil combustion, to ambient pollution in Galway, Ireland using the multilinear engine (ME-2). During periods influenced by marine air masses, local source contribution had dominant impact and nonsea-spray primary organic emissions comprised 88% of total organic aerosol mass, with peat burning found to be the greatest contributor (39%), followed by oil (21%), coal (17%), and wood (11%). In contrast, the resolved oxygenated organic aerosol (OOA) dominated the aerosol composition in continental air masses, with contributions of 50%, compared to 12% in marine air masses. The source apportionment results suggest that the use of domestic solid fuels (peat, wood, and coal) for home heating is the major source of evening and night-time particulate pollution events despite their small use.
WOS关键词	POSITIVE MATRIX FACTORIZATION ; MASS-SPECTROMETER DATA ; SOURCE APPORTIONMENT ; AIR-POLLUTION ; CHEMICAL-COMPOSITION ; CORK HARBOR ; COMBUSTION ; EMISSIONS ; COMPONENTS ; PARTICLES
WOS研究方向	Engineering ; Environmental Sciences & Ecology
语种	英语
WOS记录号	WOS:000411549800040
内容类型	期刊论文
源URL	[http://ir.ieecas.cn/handle/361006/5413]
专题	地球环境研究所_粉尘与环境研究室
作者单位	1.Paul Scherrer Inst, Lab Atmospher Chem, CH-5232 Villigen, Switzerland 2.Natl Univ Ireland Galway, Sch Phys, Univ Rd, Galway H91CF50, Ireland 3.Chinese Acad Sci, State Key Lab Loess & Quaternary Geol, Inst Earth Environm, Xian 710061, Shaanxi, Peoples R China 4.Chinese Acad Sci, Inst Earth Environm, Key Lab Aerosol Chem & Phys, Xian 710061, Shaanxi, Peoples R China 5.Univ Coll Cork, Dept Chem, Cork T23XE10, Ireland 6.Univ Coll Cork, Environm Res Inst, Cork T23XE10, Ireland 7.Natl Univ Ireland Galway, Ryan Inst, Ctr Climate & Air Pollut Studies, Univ Rd, Galway H91CF50, Ireland
推荐引用方式 GB/T 7714	O'Dowd, Colin,Huang, Ru-Jin,Prevot, Andre Stephan Henry,et al. Characterization of Primary Organic Aerosol from Domestic Wood, Peat, and Coal Burning in Ireland[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY,2017,51(18):10624-10632.
APA	O'Dowd, Colin.,Huang, Ru-Jin.,Prevot, Andre Stephan Henry.,Canonaco, Francesco.,Lin, Chunshui.,...&Ovadnevaite, Jurgita.(2017).Characterization of Primary Organic Aerosol from Domestic Wood, Peat, and Coal Burning in Ireland.ENVIRONMENTAL SCIENCE & TECHNOLOGY,51(18),10624-10632.
MLA	O'Dowd, Colin,et al."Characterization of Primary Organic Aerosol from Domestic Wood, Peat, and Coal Burning in Ireland".ENVIRONMENTAL SCIENCE & TECHNOLOGY 51.18(2017):10624-10632.