Heterogeneous reactions of mineral dust aerosol: implications for tropospheric oxidation capacity | |
Tang, Mingjin1,2; Huang, Xin3; Lu, Keding4; Ge, Maofa5; Li, Yongjie6; Cheng, Peng7; Zhu, Tong4; Ding, Aijun3; Zhang, Yuanhang4; Gligorovski, Sasho1,2 | |
刊名 | ATMOSPHERIC CHEMISTRY AND PHYSICS |
2017-10-05 | |
卷号 | 17期号:19页码:11727-11777 |
英文摘要 | Heterogeneous reactions of mineral dust aerosol with trace gases in the atmosphere could directly and indirectly affect tropospheric oxidation capacity, in addition to aerosol composition and physicochemical properties. In this article we provide a comprehensive and critical review of laboratory studies of heterogeneous uptake of OH, NO3, O-3, and their directly related species as well (including HO2, H2O2, HCHO, HONO, and N2O5) by mineral dust particles. The atmospheric importance of heterogeneous uptake as sinks for these species is assessed (i) by comparing their lifetimes with respect to heterogeneous reactions with mineral dust to lifetimes with respect to other major loss processes and (ii) by discussing relevant field and modeling studies. We have also outlined major open questions and challenges in laboratory studies of heterogeneous uptake by mineral dust and discussed research strategies to address them in order to better understand the effects of heterogeneous reactions with mineral dust on tropospheric oxidation capacity. |
语种 | 英语 |
内容类型 | 期刊论文 |
源URL | [http://ir.iccas.ac.cn/handle/121111/41082] |
专题 | 化学研究所_分子动态与稳态结构实验室 |
作者单位 | 1.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou, Guangdong, Peoples R China 2.Chinese Acad Sci, Guangzhou Inst Geochem, Guangdong Key Lab Environm Protect & Resources Ut, Guangzhou, Guangdong, Peoples R China 3.Nanjing Univ, Sch Atmospher Sci, Joint Int Res Lab Atmospher & Earth Syst Sci JirL, Nanjing, Jiangsu, Peoples R China 4.Peking Univ, Coll Environm Sci & Engn, State Key Joint Lab Environm Simulat & Pollut Con, Beijing, Peoples R China 5.Chinese Acad Sci, Inst Chem, State Key Lab Struct Chem Unstable & Stable Speci, Beijing Natl Lab Mol Sci, Beijing, Peoples R China 6.Univ Macau, Fac Sci & Technol, Dept Civil & Environm Engn, Ave Univ, Taipa, Macau, Peoples R China 7.Jinan Univ, Inst Mass Spectrometer & Atmospher Environm, Guangzhou, Guangdong, Peoples R China 8.Chinese Acad Sci, Inst Urban Environm, Ctr Excellence Reg Atmospher Environm, Xiamen 361021, Peoples R China |
推荐引用方式 GB/T 7714 | Tang, Mingjin,Huang, Xin,Lu, Keding,et al. Heterogeneous reactions of mineral dust aerosol: implications for tropospheric oxidation capacity[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2017,17(19):11727-11777. |
APA | Tang, Mingjin.,Huang, Xin.,Lu, Keding.,Ge, Maofa.,Li, Yongjie.,...&Wang, Xinming.(2017).Heterogeneous reactions of mineral dust aerosol: implications for tropospheric oxidation capacity.ATMOSPHERIC CHEMISTRY AND PHYSICS,17(19),11727-11777. |
MLA | Tang, Mingjin,et al."Heterogeneous reactions of mineral dust aerosol: implications for tropospheric oxidation capacity".ATMOSPHERIC CHEMISTRY AND PHYSICS 17.19(2017):11727-11777. |
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