In-situ carbonization approach for the binder-free Ir-dispersed ordered mesoporous carbon hydrogen evolution electrode
Zhang, Tao1; He, Yanghua1; Xu, Jinming1; Wang, Fanan1,2; Zhao, Xiaochen1; Yin, Guangzhao3; Mao, Qing3; Huang, Yanqiang1
刊名JOURNAL OF ENERGY CHEMISTRY
2017-11-01
卷号26期号:6页码:1140-1146
关键词In-situ carbonization Ordered mesoporous carbon HER
英文摘要A binder-free Ir-dispersed ordered mesoporous carbon (Ir-OMC) catalytic electrode has been prepared through a designed in-situ carbonization method, which involves coating resorcinol and formaldehyde mixtures with iridium precursors onto the three-dimensional nickel foam framework, followed by in-situ calcination in N-2 atmosphere at 800 degrees C for 3 h. This electrode shows a large surface area, ordered mesoporous structure and homogeneous distribution of metal nanoparticles. It presents good activity and stability towards hydrogen evolution reaction, which is attributed to the efficient mass and electron transport from the intimate contact among Ir nanoparticles, ordered mesoporous carbon matrix and 3D conductive substrate. We hope that this in-situ carbonization synthetic route can also be applied to design more high-performance catalysts for water splitting, fuel cells and other clean energy devices. (C) 2017 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. and Science Press. All rights reserved.
WOS标题词Science & Technology ; Physical Sciences ; Technology
类目[WOS]Chemistry, Applied ; Chemistry, Physical ; Energy & Fuels ; Engineering, Chemical
研究领域[WOS]Chemistry ; Energy & Fuels ; Engineering
关键词[WOS]MODIFIED NICKEL FOAM ; ELECTROCHEMICAL PERFORMANCE ; RESORCINOL-FORMALDEHYDE ; FACILE SYNTHESIS ; ENERGY ; CATALYSTS ; STORAGE ; ELECTROCATALYSTS ; NANOCOMPOSITE ; CONVERSION
收录类别SCI
语种英语
WOS记录号WOS:000415600300009
内容类型期刊论文
源URL[http://cas-ir.dicp.ac.cn/handle/321008/149671]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Liaoning, Peoples R China
2.Univ Chinese Acad Sci, Beijing 049, Peoples R China
3.Dalian Univ Technol, Sch Chem Engn, Dalian 116024, Liaoning, Peoples R China
推荐引用方式
GB/T 7714
Zhang, Tao,He, Yanghua,Xu, Jinming,et al. In-situ carbonization approach for the binder-free Ir-dispersed ordered mesoporous carbon hydrogen evolution electrode[J]. JOURNAL OF ENERGY CHEMISTRY,2017,26(6):1140-1146.
APA Zhang, Tao.,He, Yanghua.,Xu, Jinming.,Wang, Fanan.,Zhao, Xiaochen.,...&Huang, Yanqiang.(2017).In-situ carbonization approach for the binder-free Ir-dispersed ordered mesoporous carbon hydrogen evolution electrode.JOURNAL OF ENERGY CHEMISTRY,26(6),1140-1146.
MLA Zhang, Tao,et al."In-situ carbonization approach for the binder-free Ir-dispersed ordered mesoporous carbon hydrogen evolution electrode".JOURNAL OF ENERGY CHEMISTRY 26.6(2017):1140-1146.
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