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Microfluidic biosynthesis of silver nanoparticles: Effect of process parameters on size distribution
Liu, Hongyu ; Huang, Jiale ; Sun, Daohua ; Lin, Liqin ; Lin, Wenshuang ; Li, Jun ; Jiang, Xinde ; Wu, Weiwei ; Li, Qingbiao ; Huang JL(黄加乐)
刊名http://dx.doi.org/10.1016/j.cej.2012.08.049
2012-10-15
关键词SHAPE-CONTROLLED SYNTHESIS GOLD NANOPARTICLES METAL NANOPARTICLES LAMINAR-FLOW MICROREACTOR GROWTH LEAF NANOCRYSTALS NUCLEATION BIOREDUCTION
英文摘要Fundamental Research Funds for Central Universities [2010121051]; NSFC [21106117, 21036004, 20976146]; Research Fund for the Doctoral Program of Higher Education of China [20100121110032, 20110121120018]; NSF-Fujian Projects [2010J05032]; Here, microfluidic biosynthesis of Ag nanoparticles (AgNPs) in tubular microreactors in the presence of Cacumen Platycladi (C. Platycladi) extract was studied, focusing on the effect of technical parameters (volumetric flow rate, the concentration of C. Platycladi extract, inlet mixing pattern) and reactor parameters (reactor materials and inner diameter) on the size distribution of AgNPs. Computational fluid dynamics (CFD) was utilized to simulate the profile evolution of velocity, biomass concentration and temperature in the microreactors. It was found that, unlike in traditional bulk reactors, the interfacial effect between the solid surface and bulk solutions in microreactors could not be ignored and had crucial influence on particle size distribution. Results of CFD simulation confirmed that microchannels possessed some unique flow characteristics and various process parameters had specific influences on the size distribution of the AgNPs, which could be explained in terms of their influences on the interfacial effect and flow characteristics. Our work provides useful insight into the influence of process parameters on size distribution of AgNPs in microfluidic biosynthesis. (C) 2012 Elsevier B.V. All rights reserved.
语种英语
内容类型期刊论文
源URL[http://dspace.xmu.edu.cn/handle/2288/64390]  
专题化学化工-已发表论文
推荐引用方式
GB/T 7714
Liu, Hongyu,Huang, Jiale,Sun, Daohua,et al. Microfluidic biosynthesis of silver nanoparticles: Effect of process parameters on size distribution[J]. http://dx.doi.org/10.1016/j.cej.2012.08.049,2012.
APA Liu, Hongyu.,Huang, Jiale.,Sun, Daohua.,Lin, Liqin.,Lin, Wenshuang.,...&黄加乐.(2012).Microfluidic biosynthesis of silver nanoparticles: Effect of process parameters on size distribution.http://dx.doi.org/10.1016/j.cej.2012.08.049.
MLA Liu, Hongyu,et al."Microfluidic biosynthesis of silver nanoparticles: Effect of process parameters on size distribution".http://dx.doi.org/10.1016/j.cej.2012.08.049 (2012).
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