Impacts of Large-Scale Land-Use Change on the Uptake of Polycyclic Aromatic Hydrocarbons in the Artificial Three Northern Regions Shelter Forest Across Northern China | |
Huang, Tao; Zhang, Xiaodong; Ling, Zaili; Zhang, Leiming; Gao, Hong; Tian, Chongguo; Guo, Jiujiu; Zhao, Yuan; Wang, Li; Ma, Jianmin | |
刊名 | ENVIRONMENTAL SCIENCE & TECHNOLOGY |
2016-12-06 | |
卷号 | 50期号:23页码:12885-12893 |
ISSN号 | 0013-936X |
通讯作者 | Ma, JM (reprint author), Lanzhou Univ, Coll Earth & Environm Sci, Key Lab Environm Pollut Predict & Control, Lanzhou 730000, Gansu, Peoples R China. |
产权排序 | [Huang, Tao; Zhang, Xiaodong; Ling, Zaili; Gao, Hong; Guo, Jiujiu; Zhao, Yuan; Wang, Li; Ma, Jianmin] Lanzhou Univ, Coll Earth & Environm Sci, Key Lab Environm Pollut Predict & Control, Lanzhou 730000, Gansu, Peoples R China; [Zhang, Leiming] Environm & Climate Change Canada, Air Qual Res Div, Toronto, ON M3H 5T4, Canada; [Tian, Chongguo] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Zone Environm Proc & Ecol Remedia, Yantai 264003, Peoples R China; [Ma, Jianmin] CAS Ctr Excellence Tibetan Plateau Earth Sci, Beijing 100101, Peoples R China |
英文摘要 | This study quantifies the influence of large-scale land-use change induced by the artificial Three-Northern Regions Shelter Forest (TNRSF) across northern China on the environmental cycling of organic chemicals. Atmospheric removal and long-term trends of two polycyclic aromatic hydrocarbon (PAH) species, phenanthrene (PHE) and benzo[a]pyrene (BaP), resulting from increasing vegetation coverage and soil organic carbon in the TNRSF over the last two decades were examined. Field sampling data and modeling result showed that the total atmospheric removal of PHE by TNRSF increased from 36.4 tons in 1990 to 76.8 tons in 2010, increasing at a rate of 5.6% yr(-1), and BaP from 2.2 to 4.5 tons, increasing at a rate of 5.2% yr(-1). Three model scenarios were designed to distinguish the effects of atmospheric emissions, and with and without TNRSF on the environmental fate of PAHs. Approximately 1-4% of PHE and BaP emitted in northern China were removed by the TNRSF during 1990-2010. Model simulations revealed that the TNRSF enhanced atmospheric removal of PHE by 29% and BaP by 53% compared with the simulation without the TNRSF, manifesting marked contributions of land-use change by the artificial TNRSF, the largest afforestation activity in human history, to the atmospheric removal of organic chemicals. |
研究领域[WOS] | Engineering ; Environmental Sciences & Ecology |
关键词[WOS] | PERSISTENT ORGANIC POLLUTANTS ; GLOBAL CLIMATE-CHANGE ; POLYCHLORINATED-BIPHENYLS ; ENVIRONMENTAL FATE ; BACKGROUND SOILS ; DRY DEPOSITION ; CARBON STOCKS ; VEGETATION ; TRANSPORT ; PCBS |
收录类别 | SCI |
语种 | 英语 |
WOS记录号 | WOS:000389557100041 |
内容类型 | 期刊论文 |
源URL | [http://ir.yic.ac.cn/handle/133337/19263] |
专题 | 烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室 |
作者单位 | 1.Lanzhou Univ, Coll Earth & Environm Sci, Key Lab Environm Pollut Predict & Control, Lanzhou 730000, Gansu, Peoples R China 2.Environm & Climate Change Canada, Air Qual Res Div, Toronto, ON M3H 5T4, Canada 3.Environm & Climate Change Canada, Air Qual Res Div, Toronto, ON M3H 5T4, Canada 4.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Zone Environm Proc & Ecol Remedia, Yantai 264003, Peoples R China 5.CAS Ctr Excellence Tibetan Plateau Earth Sci, Beijing 100101, Peoples R China |
推荐引用方式 GB/T 7714 | Huang, Tao,Zhang, Xiaodong,Ling, Zaili,et al. Impacts of Large-Scale Land-Use Change on the Uptake of Polycyclic Aromatic Hydrocarbons in the Artificial Three Northern Regions Shelter Forest Across Northern China[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY,2016,50(23):12885-12893. |
APA | Huang, Tao.,Zhang, Xiaodong.,Ling, Zaili.,Zhang, Leiming.,Gao, Hong.,...&Ma, Jianmin.(2016).Impacts of Large-Scale Land-Use Change on the Uptake of Polycyclic Aromatic Hydrocarbons in the Artificial Three Northern Regions Shelter Forest Across Northern China.ENVIRONMENTAL SCIENCE & TECHNOLOGY,50(23),12885-12893. |
MLA | Huang, Tao,et al."Impacts of Large-Scale Land-Use Change on the Uptake of Polycyclic Aromatic Hydrocarbons in the Artificial Three Northern Regions Shelter Forest Across Northern China".ENVIRONMENTAL SCIENCE & TECHNOLOGY 50.23(2016):12885-12893. |
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