Synthesis and application of metal-containing ZSM-5 for the selective catalytic reduction of NOx with NH3 | |
Enhui Yuan1,4; Kun Zhang2; Lu GX(吕功煊)1; Zunli Mo3; Tang ZC(唐志诚)1 | |
刊名 | Journal of Industrial and Engineering Chemistry |
2016 | |
卷号 | 42页码:142-148 |
关键词 | NH3-SCR reaction Catalytic reduction Cu-ZSM-5 Hydrothermal stability |
ISSN号 | 1226-086X |
通讯作者 | 唐志诚 |
英文摘要 | We reported a new one-pot method to synthesize Cu incorporated ZSM-5 with ethylene diamine tetraacetic acid copper disodium salt hydrate (EDTA-Cu) as copper source by a hydrothermal process. The obtained isomorphous substituted Cu-ZSM-5 exhibits more excellent reactivity for selective catalytic reduction of NOx by NH3 with long term stability than their conventional copper impregnated counterparts. The results indicate that the tetracoordinated Cu species in the ZSM-5 frameworks have superior catalytic properties than the Cu species existed outside the ZSM-5 zeolites frameworks. The novel ammonium salt complex method was used for the first time to synthesize the metal-ZSM-5 molecular sieves. |
学科主题 | 物理化学与绿色催化 |
收录类别 | SCI |
资助信息 | Science and Technology Service Network Initiative (STS) of Chinese Academy of Science (KFJ-SW-STS-149);the National Basic Research Program of China (2013CB933200);the National Natural Science Foundation of China (21407154;21507137;21573074;21373004);the West Light Foundation of the Chinese Academy of Sciences |
语种 | 英语 |
WOS记录号 | WOS:000384873100020 |
内容类型 | 期刊论文 |
源URL | [http://210.77.64.217/handle/362003/20900] |
专题 | 兰州化学物理研究所_ERC国家工程研究中心 兰州化学物理研究所_OSSO国家重点实验室 |
作者单位 | 1.State Key Laboratory for Oxo Synthesis and Selective Oxidation, and National Engineering Research Center for Fine Petrochemical Intermediates, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou 730000, China 2.Shanghai Key Laboratory of Green Chemistry and Chemical Processes, School of Chemistry and Molecular Engineering, East China Normal University, Shanghai 200062, China 3.College of Chemistry, Northwest Normal University, Lanzhou 730070, China 4.School of Materials Science and Engineering, Nankai University, Tianjin 300071, China |
推荐引用方式 GB/T 7714 | Enhui Yuan,Kun Zhang,Lu GX,et al. Synthesis and application of metal-containing ZSM-5 for the selective catalytic reduction of NOx with NH3[J]. Journal of Industrial and Engineering Chemistry,2016,42:142-148. |
APA | Enhui Yuan,Kun Zhang,Lu GX,Zunli Mo,&Tang ZC.(2016).Synthesis and application of metal-containing ZSM-5 for the selective catalytic reduction of NOx with NH3.Journal of Industrial and Engineering Chemistry,42,142-148. |
MLA | Enhui Yuan,et al."Synthesis and application of metal-containing ZSM-5 for the selective catalytic reduction of NOx with NH3".Journal of Industrial and Engineering Chemistry 42(2016):142-148. |
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