Unveiling Microscopic Structures of Charged Water Interfaces by Surface-Specific Vibrational Spectroscopy

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	Unveiling Microscopic Structures of Charged Water Interfaces by Surface-Specific Vibrational Spectroscopy
	Wen, YC; Zha, S; Liu, X; Yang, SS; Guo, P; Shi, GS; Fang, HP; Shen, YR; Tian, CS
刊名	PHYSICAL REVIEW LETTERS
	2016
卷号	116 期号:1 页码:—
关键词	SUM-FREQUENCY GENERATION X-RAY-DIFFRACTION ABSORPTION SPECTROSCOPY ATOMIC-RESOLUTION AQUEOUS-SOLUTIONS ACID MONOLAYERS MOLECULES POLARIZATION CARBOXYLATE POTENTIALS
ISSN号	0031-9007
通讯作者	Shen, YR (reprint author), Fudan Univ, Dept Phys, State Key Lab Surface Phys, Shanghai 200433, Peoples R China.
英文摘要	A sum-frequency spectroscopy scheme is developed that allows the measurement of vibrational spectra of the interfacial molecular structure of charged water interfaces. The application of this scheme to a prototype lipid-aqueous interface as a demonstration reveals an interfacial hydrogen-bonding water layer structure that responds sensitively to the charge state of the lipid headgroup and its interaction with specific ions. This novel technique provides unique opportunities to search for better understanding of electrochemistry and biological aqueous interfaces at a deeper molecular level.
收录类别	SCI
语种	英语
WOS记录号	WOS:000367677300003
内容类型	期刊论文
源URL	[http://ir.sinap.ac.cn/handle/331007/25887]
专题	上海应用物理研究所_中科院上海应用物理研究所2011-2017年
推荐引用方式 GB/T 7714	Wen, YC,Zha, S,Liu, X,et al. Unveiling Microscopic Structures of Charged Water Interfaces by Surface-Specific Vibrational Spectroscopy[J]. PHYSICAL REVIEW LETTERS,2016,116(1):—.
APA	Wen, YC.,Zha, S.,Liu, X.,Yang, SS.,Guo, P.,...&Tian, CS.(2016).Unveiling Microscopic Structures of Charged Water Interfaces by Surface-Specific Vibrational Spectroscopy.PHYSICAL REVIEW LETTERS,116(1),—.
MLA	Wen, YC,et al."Unveiling Microscopic Structures of Charged Water Interfaces by Surface-Specific Vibrational Spectroscopy".PHYSICAL REVIEW LETTERS 116.1(2016):—.