Two-dimensional gold nanostructures with high activity for selective oxidation of carbon-hydrogen bonds | |
Wang, L; Zhu, YH; Wang, JQ; Liu, FD; Huang, JF; Meng, XJ; Basset, JM; Han, Y; Xiao, FS | |
刊名 | NATURE COMMUNICATIONS |
2015 | |
卷号 | 6页码:— |
关键词 | LAYERED DOUBLE HYDROXIDES GRAPHENE SHEETS VISIBLE-LIGHT EDGE SITES MOS2 NANOPARTICLES EVOLUTION NANOSHEETS CATALYSTS STABILIZATION |
英文摘要 | Efficient synthesis of stable two-dimensional (2D) noble metal catalysts is a challenging topic. Here we report the facile synthesis of 2D gold nanosheets via a wet chemistry method, by using layered double hydroxide as the template. Detailed characterization with electron microscopy and X-ray photoelectron spectroscopy demonstrates that the nanosheets are negatively charged and [001] oriented with thicknesses varying from single to a few atomic layers. X-ray absorption spectroscopy reveals unusually low gold-gold coordination numbers. These gold nanosheets exhibit high catalytic activity and stability in the solvent-free selective oxidation of carbon-hydrogen bonds with molecular oxygen. |
收录类别 | SCI |
语种 | 英语 |
公开日期 | 2015-12-24 |
内容类型 | 期刊论文 |
源URL | [http://ir.sinap.ac.cn/handle/331007/24615] |
专题 | 上海应用物理研究所_中科院上海应用物理研究所2011-2017年 |
推荐引用方式 GB/T 7714 | Wang, L,Zhu, YH,Wang, JQ,et al. Two-dimensional gold nanostructures with high activity for selective oxidation of carbon-hydrogen bonds[J]. NATURE COMMUNICATIONS,2015,6:—. |
APA | Wang, L.,Zhu, YH.,Wang, JQ.,Liu, FD.,Huang, JF.,...&Xiao, FS.(2015).Two-dimensional gold nanostructures with high activity for selective oxidation of carbon-hydrogen bonds.NATURE COMMUNICATIONS,6,—. |
MLA | Wang, L,et al."Two-dimensional gold nanostructures with high activity for selective oxidation of carbon-hydrogen bonds".NATURE COMMUNICATIONS 6(2015):—. |
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